To match all remaining pages and redirect to the home page of the new site you'll need to use the RedirectMatch directive (also from mod_alias). For example:
RedirectMatch 301 .* https://newdomain.com/
The RedirectMatch directive uses regex to match the request URL, whereas Redirect uses simple prefix matching.
You can't use a Redirect directive here, which is prefix matching, because whilst a redirect such as Redirect / https://newdomain.com/ will match all the remaining URLs, it will redirect to the same URL-path at newdomain.com. eg. /whatever.htm would redirect to https://newdomain.com/whatever.htm (which presumably doesn't exist - although that might actually be a good thing - since mass redirects to the home page will be seen as a soft-404 anyway by Google and a real 404 can be more informative for users).
Just to add, this does assume that newdomain.com is hosted on a different server, otherwise, you'll get a redirect loop.